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ChemicalBook CAS DataBase List Diphenyl carbonate
102-09-0

Diphenyl carbonate synthesis

12synthesis methods
Diphenyl carbonate is prepared by passing phosgene into a solution of phenol in aqueous sodium hydroxide in the presence of an inert solvent such as methylene chloride:


The organic phase, which contains the diphenyl carbonate, is separated; the solvent is stripped off and the diphenyl carbonate is purified by distillation. The reaction is accelerated by tertiary amines and is analogous to the interfacial polycondensation of 2,2-bis(4'hydroxyphenyl)propane and phosgene described. Diphenyl carbonate is a white crystalline solid, m.p. 78°C.
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Yield:102-09-0 90%

Reaction Conditions:

with 1H-imidazole;potassium carbonate at 95; under 750.075 Torr; for 9 h;Inert atmosphere;Time;

Steps:

1 Example 1
Under a nitrogen atmosphere, 7.05 g of phenol, 1.41 g of imidazole and 1.41 g of potassium carbonate were mixed in a three-necked round bottom flask equipped with a dispenser, and after the temperature of the oil bath reached 95 ° C,Add 13.5 g of dimethyl carbonate (molar ratio of phenol, imidazole, potassium carbonate and dimethyl carbonate: 1:0.28:0.14:2), and react under normal pressure (0.1 MPa) for 9 hours, while passing through the reaction. A simple distillation method vaporizes the produced methanol and its azeotrope to a dispenser and removes it. At the end of the reaction, the catalyst is recovered and the solution is carried out. By gas chromatography, the phenol conversion was 38.9%, the selectivity to diphenyl carbonate was 90.5%, and the methyl phenyl carbonate (MPC) was selected to be 3.5%.

References:

Sinopec Corporation;Sinopec Corporation Beijing Chemical Institute;Xie Lunjia;Wang Dawei;Liu Qing;Li Wei CN108727192, 2018, A Location in patent:Paragraph 0054-0067

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