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ChemicalBook CAS DataBase List 1-Boc-4-[methoxy(methyl)carbamoyl]piperidine
139290-70-3

1-Boc-4-[methoxy(methyl)carbamoyl]piperidine synthesis

11synthesis methods
6638-79-5 Synthesis
N,O-Dimethylhydroxylamine hydrochloride

6638-79-5
573 suppliers
$6.00/25g

84358-13-4 Synthesis
N-BOC-piperidine-4-carboxylic acid

84358-13-4
389 suppliers
$5.00/5g

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Yield: 100%

Reaction Conditions:

Stage #1:N,O-dimethylhydroxylamine*hydrochloride;N-[(tert-butoxy)carbonyl]piperidine-4-carboxylic acid with triethylamine in DMF (N,N-dimethyl-formamide) at 20; for 0.166667 h;
Stage #2: with benzotriazol-1-ol;1-ethyl-(3-(3-dimethylamino)propyl)-carbodiimide hydrochloride in DMF (N,N-dimethyl-formamide)
Stage #3: with hydrogenchloride in water

Steps:

3
To a stirring suspension of t-Boc-isonipecotic acid (19) (2.34 g, 10.2 mmol) and the Weinreb amine (1.5 g, 15 mmol) in DMF (50 mL), was added triethylamine (2.8 mL, 20 mmol) at room temperature. After stirring for 10 min, HOBt (1.62 g, 12 mmol) was added, followed by EDCI (2.3 g, 12 mmol). The resulting solution was stirred overnight and concentrated. The residue was taken up in 1 N HCl (100 mL) and extracted with EtOAc (3×100 mL). The combined organic extracts were washed with sat NaHCO3 (50 mL), brine (50 mL), dried (MgSO4) and concentrated to obtain a colorless oil (20) (2.79 g, >100%). 1H NMR (500 MHz, CDCL3) δ4.14 (m, 2H), 3.71 (s, 3H), 3.19 (s, 3H), 2.78 (m, 3H), 1.68 (m, 4H), 1.46 (s, 9H); MS (ESI+) m/z 217.72 (M+H+-isobutylene).

References:

Myriad Pharmaceuticals, Inc. US2004/14763, 2004, A1 Location in patent:Page 21

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