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Density Functional Theory Study on the Selective Reductive Amination of Aldehydes and Ketones over Their Reductions to Alcohols Using Sodium Triacetoxyborohydride
10.1021/acsomega.2c04056
ACS Omega
American Chemical Society
Shannon J. Oliphant (ORCID: g/0000-0003-1327-7300)
Robert H. Morris (ORCID: g/0000-0002-7574-9388)
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http://pubs.acs.org/doi/suppl/10.1021/acsomega.2c04056
© 2022 The Authors - License: © 2022 The Authors. Published by American Chemical Society
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(\n \r)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 239.924 314.816 cm
BT
/F9 1 Tf
0.0252 Tc
1 TL
0 0 Td
(')Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
1 j
1 J
0 w
10 0 0 10 250.639 310.394 cm
BT
/F9 1 Tf
0.0189 Tc
1 TL
0 0 Td
(\r\r)Tj
0 Tc
-19.916 -1.1111 Td
( )Tj
4.4957 0 Td
( \n \r)Tj
6.9335 0 Td
( )Tj
2.931 0 Td
(%)Tj
4.6771 0 Td
()Tj
1.3775 0 Td
( )Tj
1.4911 0 Td
(\))Tj
/F2 1 Tf
()Tj
/F9 1 Tf
(/)Tj
-21.9059 -1.1112 Td
(%\n)Tj
5.7713 0 Td
( \r)Tj
3.9288 0 Td
( )Tj
1.6497 0 Td
(\n)Tj
4.4844 0 Td
( )Tj
1.5647 0 Td
()Tj
4.0081 0 Td
( \n %)Tj
-21.407 -1.1112 Td
()Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 68.7118 281.48 cm
BT
/F9 1 Tf
1 TL
0 0 Td
(0)Tj
/C3 cs 0 0 0 scn
()Tj
/C3 cs 0.05 0.33 0.65 scn
(1)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
1 j
1 J
0 w
10 0 0 10 84.0755 277.058 cm
BT
/F9 1 Tf
1 TL
0 0 Td
()Tj
1.4853 0 Td
( )Tj
3.6113 0 Td
()Tj
1.8765 0 Td
( )Tj
3.7417 0 Td
(\r)Tj
3.0955 0 Td
()Tj
2.3357 0 Td
( )Tj
-19.4058 -1.1111 Td
()Tj
3.6169 0 Td
( )Tj
0.8391 0 Td
( )Tj
3.719 0 Td
(\n)Tj
4.5524 0 Td
( )Tj
1.8368 0 Td
( )Tj
1.3437 0 Td
( \n)Tj
2.7495 0 Td
(\n)Tj
4.5525 0 Td
()Tj
-23.2099 -1.1112 Td
(\n)Tj
2.2224 0 Td
( )Tj
1.2981 0 Td
(\n)Tj
2.744 0 Td
()Tj
2.6645 0 Td
(\r)Tj
0.9751 0 Td
()Tj
2.1033 0 Td
()Tj
3.4412 0 Td
()Tj
1.1793 0 Td
( )Tj
1.2982 0 Td
( )Tj
3.7531 0 Td
( \n)Tj
-21.6792 -1.1112 Td
()Tj
3.5205 0 Td
()Tj
/C3 cs 0.05 0.33 0.65 scn
(\n)Tj
3.9175 0 Td
(&)Tj
/C3 cs 0 0 0 scn
(#)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 136.743 248.145 cm
BT
/F9 1 Tf
1 TL
0 0 Td
(2)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
1 j
1 J
0 w
10 0 0 10 145.757 243.723 cm
BT
/F9 1 Tf
1 TL
0 0 Td
(\()Tj
2.9253 0 Td
()Tj
4.0422 0 Td
( \n )Tj
4.5637 0 Td
()Tj
-20.9591 -1.1111 Td
(\n )Tj
4.0251 0 Td
()Tj
1.0148 0 Td
()Tj
1.4741 0 Td
(\n)Tj
2.4094 0 Td
( )Tj
1.6666 0 Td
(\r\r,)Tj
4.5411 0 Td
()Tj
3.9231 0 Td
()Tj
2.3755 0 Td
()Tj
0.9978 0 Td
(\r)Tj
-22.4275 -1.1169 Td
(\r\r)Tj
3.5659 0 Td
( )Tj
0.8391 0 Td
()Tj
4.6261 0 Td
(%)Tj
3.4071 0 Td
(\r\r\r)Tj
3.8438 0 Td
(\n)Tj
3.3845 0 Td
()Tj
1.2189 0 Td
()Tj
-20.8854 -1.1111 Td
( )Tj
3.7077 0 Td
( \n\r)Tj
3.2088 0 Td
(3)Tj
2.7891 0 Td
(\r)Tj
2.3131 0 Td
( )Tj
3.4242 0 Td
(\r)Tj
4.5468 0 Td
()Tj
1.5533 0 Td
()Tj
-21.543 -1.1112 Td
()Tj
1.1565 0 Td
()Tj
3.7077 0 Td
( )Tj
2.4605 0 Td
(\r)Tj
0.9864 0 Td
( )Tj
2.8969 0 Td
( \r)Tj
1.1509 0 Td
()Tj
0.9354 0 Td
(\n\r)Tj
2.279 0 Td
(\r)Tj
4.2576 0 Td
()Tj
2.9594 0 Td
()Tj
-22.7903 -1.1112 Td
(\n)Tj
2.5682 0 Td
()Tj
2.0749 0 Td
()Tj
1.6271 0 Td
( )Tj
3.6962 0 Td
(\n)Tj
4.5354 0 Td
(\r )Tj
3.2599 0 Td
(\n )Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 261.865 192.586 cm
BT
/F9 1 Tf
1 TL
0 0 Td
(4)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
1 j
1 J
0 w
10 0 0 10 269.745 188.107 cm
BT
/F9 1 Tf
1 TL
0 0 Td
( \r)Tj
-21.8266 -1.1111 Td
(\r\n)Tj
3.1294 0 Td
( )Tj
8.7194 0 Td
( !"#)Tj
3.4355 0 Td
(\r)Tj
0.9014 0 Td
( )Tj
0.7257 0 Td
( )Tj
3.2372 0 Td
()Tj
2.7721 0 Td
()Tj
-22.9207 -1.1112 Td
()Tj
3.566 0 Td
( )Tj
2.3187 0 Td
( \r)Tj
1.0091 0 Td
()Tj
0.7881 0 Td
(\r\r)Tj
2.5738 0 Td
(\r)Tj
3.9968 0 Td
()Tj
1.338 0 Td
(\n\r)Tj
2.7496 0 Td
()Tj
1.9162 0 Td
( \r)Tj
-20.2563 -1.1112 Td
( )Tj
1.8142 0 Td
(\r)Tj
3.5319 0 Td
()Tj
2.7383 0 Td
()Tj
2.4378 0 Td
()Tj
3.719 0 Td
( \r)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 219.969 159.25 cm
BT
/F9 1 Tf
1 TL
0 0 Td
(4)Tj
/C3 cs 0 0 0 scn
()Tj
/C3 cs 0.05 0.33 0.65 scn
(5)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
1 j
1 J
0 w
10 0 0 10 232.781 154.772 cm
BT
/F9 1 Tf
1 TL
0 0 Td
( \r)Tj
2.1316 0 Td
(\r)Tj
-20.2618 -1.1111 Td
()Tj
1.3152 0 Td
(\n\r)Tj
2.7269 0 Td
( \r)Tj
1.4854 0 Td
()Tj
2.0636 0 Td
()Tj
3.719 0 Td
()Tj
0.9751 0 Td
(\n )Tj
2.3244 0 Td
(\r\r\r)Tj
3.6509 0 Td
(\r)Tj
4.0082 0 Td
(\r)Tj
0.0035 Tc
-22.2687 -1.1112 Td
( \r)Tj
1.4286 0 Td
()Tj
3.0954 0 Td
()Tj
2.4265 0 Td
( \r)Tj
3.4469 0 Td
()Tj
1.7575 0 Td
( )Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 212.542 136.97 cm
BT
/F9 1 Tf
0.0047 Tc
1 TL
0 0 Td
(6)Tj
/C3 cs 0 0 0 scn
()Tj
/C3 cs 0.05 0.33 0.65 scn
(7)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
1 j
1 J
0 w
10 0 0 10 228.019 132.548 cm
BT
/F9 1 Tf
0.0035 Tc
1 TL
0 0 Td
( )Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 263.339 136.97 cm
BT
/F9 1 Tf
0.0047 Tc
1 TL
0 0 Td
(&8)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
1 j
1 J
0 w
10 0 0 10 277.342 132.548 cm
BT
/F9 1 Tf
0.0035 Tc
1 TL
0 0 Td
( )Tj
0 Tc
-22.5863 -1.1111 Td
( \n)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 100.12 125.858 cm
BT
/F9 1 Tf
1 TL
0 0 Td
(&&)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
1 j
1 J
0 w
10 0 0 10 111.061 121.436 cm
BT
/F9 1 Tf
1 TL
0 0 Td
()Tj
2.6418 0 Td
( )Tj
1.2416 0 Td
(\r)Tj
1.6214 0 Td
()Tj
3.8778 0 Td
( \n )Tj
4.2009 0 Td
()Tj
3.5489 0 Td
( )Tj
-23.0907 -1.1111 Td
( )Tj
3.7643 0 Td
( )Tj
1.7745 0 Td
( )Tj
0.7766 0 Td
(\n )Tj
3.3392 0 Td
( \n)Tj
2.6872 0 Td
( )Tj
1.0715 0 Td
()Tj
1.7802 0 Td
(\r)Tj
1.9218 0 Td
()Tj
1.1226 0 Td
()Tj
2.1429 0 Td
(\r\r\r)Tj
0.0081 Tc
-20.3808 -1.1112 Td
( )Tj
2.2507 0 Td
(\r)Tj
4.5012 0 Td
()Tj
4.2406 0 Td
()Tj
1.6101 0 Td
( !")Tj
3.0161 0 Td
(\r)Tj
1.2699 0 Td
(\r )Tj
4.7111 0 Td
()Tj
1.4797 0 Td
()Tj
0 Tc
-23.0794 -1.1112 Td
( )Tj
4.1782 0 Td
()Tj
1.2246 0 Td
()Tj
1.6439 0 Td
()Tj
2.3925 0 Td
( )Tj
3.2825 0 Td
(\r)Tj
3.2144 0 Td
( \r)Tj
1.1906 0 Td
()Tj
2.0749 0 Td
( )Tj
1.7462 0 Td
(\r )Tj
-20.9478 -1.1111 Td
()Tj
1.61 0 Td
(")Tj
/F2 1 Tf
()Tj
/F9 1 Tf
($)Tj
2.4095 0 Td
()Tj
2.3866 0 Td
( )Tj
1.4684 0 Td
(\r)Tj
2.4321 0 Td
(\r)Tj
3.804 0 Td
( )Tj
1.8085 0 Td
(% )Tj
-15.9191 -1.1112 Td
(9\r)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 77.4425 70.2992 cm
BT
/F9 1 Tf
1 TL
0 0 Td
(&')Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
1 j
1 J
0 w
10 0 0 10 87.4771 65.8771 cm
BT
/F9 1 Tf
1 TL
0 0 Td
($)Tj
3.9514 0 Td
()Tj
1.0658 0 Td
()Tj
1.5874 0 Td
()Tj
4.5695 0 Td
()Tj
2.2336 0 Td
(\r)Tj
0.8618 0 Td
()Tj
1.2755 0 Td
()Tj
2.6249 0 Td
()Tj
1.0205 0 Td
()Tj
-22.7903 -1.1111 Td
( )Tj
3.7416 0 Td
( )Tj
1.7971 0 Td
(\n )Tj
6.4573 0 Td
(\r)Tj
2.8687 0 Td
()Tj
1.5137 0 Td
(\r)Tj
4.0421 0 Td
()Tj
1.0659 0 Td
( !")Tj
4.9095 29.3836 Td
($)Tj
3.1635 0 Td
(\r)Tj
3.0387 0 Td
( )Tj
4.1215 0 Td
()Tj
2.7666 0 Td
(\(: #)Tj
2.9991 0 Td
(\n\r)Tj
3.6056 0 Td
( )Tj
1.4627 0 Td
(\r)Tj
2.0579 0 Td
()Tj
-23.2156 -1.1055 Td
( )Tj
2.9537 0 Td
()Tj
1.8652 0 Td
()Tj
4.1159 0 Td
( )Tj
4.8869 0 Td
()Tj
1.4059 0 Td
(\n)Tj
2.8063 0 Td
()Tj
4.3087 0 Td
()Tj
-22.3426 -1.1055 Td
( \r)Tj
4.0762 0 Td
( )Tj
1.7348 0 Td
(\r)Tj
3.2542 0 Td
( )Tj
1.4003 0 Td
( !")Tj
-9.5641 -1.0998 Td
(\)\n )Tj
6.1058 0 Td
(\r\r)Tj
2.9764 0 Td
()Tj
1.0885 0 Td
()Tj
1.559 0 Td
( )Tj
3.7871 0 Td
( )Tj
2.9423 0 Td
()Tj
1.1339 0 Td
()Tj
-20.4944 -1.0999 Td
( \n )Tj
4.2293 0 Td
( )Tj
2.8743 0 Td
(\r)Tj
2.3924 0 Td
()Tj
1.389 0 Td
( \r)Tj
4.0308 0 Td
(\n )Tj
2.5002 0 Td
( \r\r)Tj
3.4979 0 Td
( )Tj
1.8028 0 Td
()Tj
-22.7167 -1.1055 Td
(\r\r )Tj
4.3483 0 Td
(\n\n)Tj
4.3427 0 Td
(\r)Tj
2.0296 0 Td
(\r)Tj
3.7077 0 Td
(\r)Tj
4.0478 0 Td
(\(: )Tj
2.1657 0 Td
( \r)Tj
1.5307 0 Td
()Tj
-22.1725 -1.0998 Td
(\r)Tj
2.0296 0 Td
()Tj
1.0658 0 Td
()Tj
2.5002 0 Td
()Tj
1.4853 0 Td
(\n \r\n\r)Tj
4.9436 0 Td
()Tj
1.0318 0 Td
()Tj
3.7871 0 Td
( \n )Tj
4.1045 0 Td
()Tj
0.0215 Tc
-20.9479 -1.1055 Td
( )Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 342.198 275.811 cm
BT
/F9 1 Tf
0.0286 Tc
1 TL
0 0 Td
(&0)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
1 j
1 J
0 w
10 0 0 10 356.712 271.389 cm
BT
/F9 1 Tf
0.0215 Tc
1 TL
0 0 Td
()Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 382.677 275.811 cm
BT
/F9 1 Tf
0.0286 Tc
1 TL
0 0 Td
(&1)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
1 j
1 J
0 w
10 0 0 10 397.247 271.389 cm
BT
/F9 1 Tf
0.0215 Tc
1 TL
0 0 Td
(\n)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 428.769 275.811 cm
BT
/F9 1 Tf
0.0286 Tc
1 TL
0 0 Td
(&2)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
1 j
1 J
0 w
10 0 0 10 443.282 271.389 cm
BT
/F9 1 Tf
0.0215 Tc
1 TL
0 0 Td
(\r\n\n)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 477.524 275.811 cm
BT
/F9 1 Tf
0.0286 Tc
1 TL
0 0 Td
(&4)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
1 j
1 J
0 w
10 0 0 10 492.094 271.389 cm
BT
/F9 1 Tf
0.0215 Tc
1 TL
0 0 Td
( )Tj
2.1543 0 Td
(\n)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 547.994 275.811 cm
BT
/F9 1 Tf
0.0286 Tc
1 TL
0 0 Td
(&5)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
1 j
1 J
0 w
10 0 0 10 315.439 260.334 cm
BT
/F9 1 Tf
0.0051 Tc
1 TL
0 0 Td
( \r\r)Tj
4.0875 0 Td
( \r)Tj
3.016 0 Td
(\r\r)Tj
3.3335 0 Td
(\r)Tj
2.6873 0 Td
()Tj
1.6724 0 Td
(\n\r)Tj
6.0604 0 Td
( \r\r)Tj
0 Tc
-20.8571 -1.0998 Td
()Tj
3.6453 0 Td
(\n )Tj
4.3426 0 Td
()Tj
4.1896 0 Td
( \r)Tj
1.3436 0 Td
()Tj
1.8028 0 Td
()Tj
3.9005 0 Td
( )Tj
2.8573 0 Td
( )Tj
-22.0817 -1.1055 Td
(\n)Tj
2.1656 0 Td
()Tj
1.542 0 Td
(\n)Tj
3.1068 0 Td
( )Tj
1.7405 0 Td
(\r\n\n)Tj
3.4015 0 Td
( \r)Tj
3.1408 0 Td
(\r\r)Tj
3.1634 0 Td
(" \r)Tj
/F10 1 Tf
3.1748 0 Td
()Tj
0.9581 0 Td
()Tj
/F9 1 Tf
()Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 548.22 242.759 cm
BT
/F9 1 Tf
1 TL
0 0 Td
(&2)Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
1 j
1 J
0 w
10 0 0 10 315.439 227.282 cm
BT
/F9 1 Tf
1 TL
0 0 Td
( )Tj
3.5319 0 Td
(\n% )Tj
6.7974 0 Td
()Tj
3.7588 0 Td
( \n )Tj
4.0818 0 Td
()Tj
1.9219 0 Td
( )Tj
1.1565 0 Td
( )Tj
-21.2483 -1.1055 Td
( )Tj
4.1952 0 Td
(\n \r\n)Tj
4.9493 0 Td
()Tj
1.4229 0 Td
()Tj
3.515 0 Td
( )Tj
1.0431 0 Td
()Tj
3.5376 0 Td
(\r)Tj
3.3166 0 Td
()Tj
-21.9797 -1.0998 Td
(; )Tj
/F10 1 Tf
4.7735 0 Td
()Tj
0.9637 0 Td
()Tj
/F9 1 Tf
()Tj
ET
Q
q
8.9575 8.9575 589.493 782.986 re
W* n
/C3 cs 0.05 0.33 0.65 scn
1 j
1 J
0 w
7.4999 0 0 6.6659 381.6 209.65 cm
BT
/F9 1 Tf
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