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Palladium-catalyzed dearomative 1, 4-hydroamination
Gilbert, Robert ; Davis, Christopher W ; Bingham, Tanner W , et al. Tetrahedron,2024,134135. DOI: 10.1016/j.tet.2024.134135
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Abstract: A dearomative 1,4-hydroamination of nonactivated arenes has been developed, using a key arene-arenophile photocycloaddition strategy to disrupt aromaticity. Palladium catalysis with K-Selectride? as a hydride source uniquely enables selective reactivity and provides access to a range of substituted 1,4-cyclohexadienes from aromatic starting materials. We demonstrate a few synthetic applications of this scalable procedure by preparing highly-functionalized small molecules in three to four steps from naphthalene.
Keywords: Dearomatization ; Hydroamination ; Arenophiles ; Palladium ; Catalysis
Purchased from AmBeed: 32005-36-0 ; 657408-07-6 ; 787618-22-8 ; 213697-53-1 ; 12150-46-8
CAS No. : | 213697-53-1 | MDL No. : | MFCD02183572 |
Formula : | C26H36NP | Boiling Point : | No data available |
Linear Structure Formula : | P(C6H11)2(C12H8(N(CH3)2)) | InChI Key : | ZEMZPXWZVTUONV-UHFFFAOYSA-N |
M.W : | 393.54 | Pubchem ID : | 2734217 |
Synonyms : |
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Chemical Name : | 2'-(Dicyclohexylphosphino)-N,N-dimethyl-[1,1'-biphenyl]-2-amine |
Signal Word: | Warning | Class: | |
Precautionary Statements: | P261-P305+P351+P338 | UN#: | |
Hazard Statements: | H315-H319-H335 | Packing Group: | |
GHS Pictogram: |